Journal article

Tensile Control of Vibrational Strong Light-Matter Coupling with Flexible Polyester Films

Goekalp Engin Akinoglu, Dali Quan, Eliza Rokhsat, James Andell Hutchison

Advanced Functional Materials | Wiley | Published : 2024

Abstract

Polaritons are generated by strong interaction between photons and matter, with the hybridization fundamentally changing the energy landscape of the system. Future exploitation of polaritons will benefit from implementing low-cost, flexible, and easily tuneable configurations, as electronics have before. Here, coherent coupling of the carbonyl stretch vibrations of polyester (poly(ethylene terephthalate), PET) films to the optical modes of a Fabry–Perot (FP) cavity is presented, in which the FP cavity is directly formed on flexible, free-standing, and commercially available PET films. For 2-µm thick PET films, the carbonyl stretch vibration of the PET overlaps with the half-wavelength FP cav..

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University of Melbourne Researchers

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Funding Acknowledgements

This work was partly performed at the Materials Characterisation and Fabrication Platform (MCFP) at the University of Melbourne and the Victorian Node of the Australian National Fabrication Facility (ANFF). The authors thank funding from the Australian Government through the Centre of Excellence in Exciton Science (CE170100026) and Discovery Project (DP160102754) and thank funding from the ANFF-Vic Technology Fellow Ambassador Program and the MCFP Sustainability Research Grant. J.A.H. thanks the Australian Government for funding through the Australian Research Council Future Fellowship scheme (FT180100295) and G.E.A. thanks funding through the Australian Government Research Training Program (RTP) Scholarship program.